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Single-molecule spectroscopy with 27 fs pulses: Time-resolved experiments and direct imaging of orientational distributions

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Abstract

Confocal microscopy of single molecules bound on a silica surface is performed with precompressed 27 fs laser pulses. Interferometric autocorrelation using a single molecule is demonstrated. It is also shown that orientational distributions can be directly obtained from one- and two-photon images produced with circularly polarized light.

Original languageEnglish (US)
Pages (from-to)7-9
Number of pages3
JournalApplied Physics Letters
Volume73
Issue number1
DOIs
StatePublished - 1998
Externally publishedYes

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy (miscellaneous)

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