Achieving ground-state polar molecular condensates by chainwise atom-molecule adiabatic passage

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Abstract

We generalize the idea of chainwise stimulated Raman adiabatic passage (STIRAP) to a photoassociation-based chainwise atom-molecule system, with the goal of directly converting two-species atomic Bose-Einstein condensates (BEC) into a ground polar molecular BEC. We pay particular attention to the intermediate Raman laser fields, a control knob inaccessible to the usual three-level model. We find that an appropriate exploration of both the intermediate laser fields and the stability property of the atom-molecule STIRAP can greatly reduce the power demand on the photoassociation laser, a key concern for STIRAPs starting from free atoms due to the small Franck-Condon factor in the free-bound transition.

Original languageEnglish (US)
Article number013632
JournalPhysical Review A - Atomic, Molecular, and Optical Physics
Volume81
Issue number1
DOIs
StatePublished - Jan 29 2010

All Science Journal Classification (ASJC) codes

  • Atomic and Molecular Physics, and Optics

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